Heteroatom-assisted olefin polymerization by rare-earth metal catalysts

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Heteroatom-assisted olefin polymerization by rare-earth metal catalysts

Heteroatom-functionalized polyolefins are of fundamental interest and practical importance. This has spurred investigations of the copolymerization of polar and nonpolar olefins. We report the first syndiospecific polymerization of a series of heteroatom-containing α-olefins and their copolymerization with ethylene catalyzed by half-sandwich rare-earth complexes. We have found that the interact...

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Group 3 metal catalysts for ethylene and -olefin polymerization

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Olefin Metathesis by Supported Metal Oxide Catalysts

The literature of olefin metathesis by heterogeneous supported catalysts, both industrial-type supported metal oxides (ReOx/Al2O3, ReOx/(SiO2−Al2O3), MoOx/SiO2, MoOx/Al2O3, MoOx/(SiO2−Al2O3), WOx/SiO2, and WOx/ (SiO2−Al2O3)) and supported organometallic complexes, is comprehensively reviewed. The focus of this Review is supported metal oxide catalysts, but the well-defined supported organometal...

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Polyolefins are of vast economic importance, which is reflected by an annual production of more than 70 million tons of polyethylene and polypropylene. While the major portion of these materials is produced with Zieglerand chromium-based catalysts, the older free-radical process that affords low-density polyethylene (LDPE) has maintained its significance.[1] Despite the necessity of working at ...

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Surface science of single-site heterogeneous olefin polymerization catalysts.

This article reviews the surface science of the heterogeneous olefin polymerization catalysts. The specific focus is on how to prepare and characterize stereochemically specific heterogeneous model catalysts for the Ziegler-Natta polymerization. Under clean, ultra-high vacuum conditions, low-energy electron irradiation during the chemical vapor deposition of model Ziegler-Natta catalysts can be...

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ژورنال

عنوان ژورنال: Science Advances

سال: 2017

ISSN: 2375-2548

DOI: 10.1126/sciadv.1701011